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    High Precision Measurements for fundamental Physics





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We are part of the group of Prof. T. W. Hänsch and located at the Max-Planck Institute for Quantum Optics Garching/Germany.MPQ-Logo






Atomic Hydrogen

The hydrogen atom is the simplest of all atoms and can therefore be treated theoretically with the utmost precision. The underlying theory is quantum electrodynamics (QED) that currently allows to determine energy levels with 12 significant digits of accuracy. To fully exploit this capability, that no other physical theory can provide, we are determined to provide experimental data that are at least as accurate. Currently the best measured quantity is the sharpest of all transitions of the hydrogen atom, which is the dipole forbidden 1S-2S transitions whose frequency we determined to be:



When comparing with the theoretical expression one finds that it contains two terms that contribute about equally to its uncertainty. This means not only the Rydberg constant that sets the scale for all atomic energy levels can be determined from such a comparison but it also that at least two measurements have to be used. However, the best analysis is to combine with all other transition frequencies that have been measured, many of them provided by the group of Francoise Biraben at the Laboratoire Kastler Brossel Paris. In this way the Rydberg constant



is fixed as one of the most accurately known fundamental constants. It's value is used for expample to derive a value for the fine structure constant alpha from independent determinations of the electrons mass devided by Planck's constant. This method has the potential to convert all digits since the of the speed of light has a defined (exact) value within the SI systen of unit.

Traditionaly the comparision with the results of quantum electrodynamics (QED) is done by using only small fraction of the energy levels called the Lamb shift which is roughly the deviation of QED from its precessing theory by Dirac. The largest of these Lamb shifts is the one of the 1s level that is determined to be



from the world experimetal data. Because at least two hydrogen transition frequencies enter to determine the two esults above, the second most precise measurement is limiting the overall accuracy. The 1S-2S transition frequency is known with almost 14 digits of accuracy while all other transition frequencies have been measured with much lower accuracy. This is the one motivation for our eforts on the 1S-3S transition frequency as explained below.

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The 1S-2S Transition

In the 1S-2S experiment hydrogen atoms are excited by longitudinal Doppler-free two photon excitation at 243nm. This radiation is generated by a frequency doubled ultra stable dye laser at 486nm. The UV radiation is then resonantly enhanced in a linear cavity inside a vacuum chamber. Atomic hydrogen from a gas discharge is directed through a nozzle cooled with liquid helium. The cold atomic beam is oriented along the axis of the enhancement resonator. After the atoms have passed some distance, usually around 10cm, a small electric field that mixes the metastable 2S state (lifetime 1/7 sec) with the fast decaying 2P state is applied. This releases a Lyman alpha photon which is registered with a photo multiplier tube. To reduce the residual second order Doppler-effect we use a delayed detection scheme where the fluorescence at 121nm is detected only after the exciting light has been switched off for some period of time, typically between 0.5 and 1.8ms. In this way we set an upper limit on the second order Doppler-shift below 1kHz.

The 1s2s hydrogen spectrometer

Part of the 486nm radiation from the ultra stable dye laser is transfered to a frequency comb to determine its frequency with the help of a GPS disciplined hydrogen maser or a Cs atomic clock. Besides the determination of the Rydberg constant and testing QED, another application is the search for a possible slow temporal variations of the fundamental constants that is suggested by some philosophical arguments.

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pdf


The 1S-3S Transition

As pointed out above, results derived from a set of hydrogen transition frequencies, will be limited in accuracy by the second most precise determination of these transitions. Therefore a measurement of another frequency besides the 1S-2S transition frequency within 14 digits of accuracy would significantly reduce the uncertainty of the Rydberg constant and the Lamb shifts. As QED allows to convert the Lamb shifts of any level into the Lamb shift of any other with very small uncertainty, it does not really matter which of the transition frequencies is used to complement the 1S-2S frequency. The right choice should therefore take the experimental simplicity, the sensitivity to systematic shifts and the line width into account. We have been trying to detect the 1S-3S transition signal not only for these reasons but also because we want to further develop direct frequency comb spectroscopy. The required wavelength of 205nm is very close to the short wavelength cut-off for second harmonic generation in beta barium borate (BBO). The crystal is highly susceptible for unwanted non-linear effects such as photo refractivity that has so far prevented its use with continuous wave lasers. In our experiment we want to use a pulsed mode locked laser instead. Such a laser posses a comb like spectrum with narrow band modes that can be used in pairs for two photon excitation. It has been shown by E.V.Baklanov and V.P.Chebotayev already in the 1970s, that with such a frequency comb excitation the effective excitation rate derives from the intensity of all modes together while the line width can be as narrow as that of a single mode of the frequency comb. To explore these possibilities could proof very useful when much shorter wavelengths are required, for example for the excitation of the 1S-2S transition in hydrogen like helium.


The 2S Hyperfine Splitting

The frequency of the 2S hyperfine interval is one of the best measured quantities in physics with about 13 digits known. The hyperfine interaction depends largely on the structure of the nucleus that can not be calculated from first principles with the required accuracy. Therefore the 2S hyperfine interval can not be used directly to test quantum electrodynamics. However, if combined with 8 times the hyperfine splitting of the 2S state according to

an accurately calculable quantity is obtained. For this combination most of the difficult to calculate terms cancel thanks to the approximate scaling of the hyperfine structure with the inverse cube of the principle quantum number. The test of quantum electrodynamics via the above difference is limited by the experimental value for the 2S hyperfine interval. Traditionally this has been measured within the radio frequency domain so that uncertainties in the optical frequencies would cancel out. Meanwhile our spectrometer is sufficiently accurate improve on these measurements with laser excitation. 

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Narrow Linewidth Lasers

To probe narrow transitions in atomic hydrogen one prerequisite is a laser whose line width is even narrower. For this reason we stabilize our spectroscopy lasers to high finesse cavities that are immunized and isolated from external perturbations such as temperature variations and vibrations. To compensate for thermal drifts the cavity spacers, that hold the mirrors apart, are made from ultralow expansion (ULE) glass which possesses a zero linear thermal expansion coefficient. A design using Peltier elements in vacuum allows operation at an optimal temperature where the quadratic temperature expansion of ULE could be eliminated as well. The spacers are mounted vertically and suspended in midplane such that the influence of vertical vibrations to the mirror separation is significantly suppressed. This makes the setup virtually immune for vertical vibrations that are more difficult to isolate than horizontal vibrations. We achieve a finesse of up to 400,000 with a drift of the optical frequency of 0.06Hz per seconod limited by material aging.The short term stability is dominated by thermally induced fluctuations of the mirror surface position. Nevertheless a laser line width of 0.5Hz has been measured by comparing two of these cavities in our lab. 

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Atomic Clocks

To generate the time base for our experiments we operate a clock system that consists of an active hydrogen maser, a cesium atomic clock, two GPS receivers and a computer for monitoring an steering. The complete system is connected to an uninterruptible power supply and is located an a quite room with very good temperature stability. We calibrate the maser by comparing it with the time signals broad casted by GPS. Comparing our data with similar data generated at the Physikalisch Technische Bundesanstalt at Braunschweig (PTB) allows us to calibrate our maser relative to the PTB clocks. A frequency comb is used to convert the masers reference frequency into the optical and distribute is via a fiber network throughout the institute.



last change Sptember 18 2008